Biden recently said that only India among the Quad group of countries was "somewhat shaky" in acting against Russia.
Lured by steep discounts following Western sanctions on Russian entities, India has bought at least 13 million barrels of Russian crude oil since the invasion in late February. That compared with some 16 million barrels for the whole of last year, data compiled by Reuters shows.
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Psaki did not disclose whether India had made any commitments on energy imports but said Washington stands ready to help the country diversify its sources of energy.
Noting Modi’s statements about the war on Monday, Psaki said, "part of our objective now is to build on that and to encourage them to do more. And that’s why it’s important to have leader to leader conversations."
A U.S. official added that "we haven’t asked India to do anything in particular." The official said "India is gonna make its own judgments" following "a very candid conversation."
Talks in Washington on Monday took place between U.S. Secretary of State Antony Blinken, U.S. Secretary of Defense Lloyd Austin and their Indian counterparts Jaishankar and Indian Defense Minister Rajnath Singh.
Blinken said India’s ties with Russia developed over decades at a time when the United States was not able to be a partner to India, but that times had since changed.
"Today we are able and willing to be a partner of choice with India across virtually every realm," Blinken said at a joint presser following the talks.
India’s modernization needs on defense were a key topic the two sides have discussed at length, the ministers said.
U.S. Defense Secretary Lloyd Austin said the two countries had signed a bilateral agreement to support sharing information and cooperation in space.
Biden told Modi he looked forward to seeing him in Japan for a Quad meeting "on about the 24th of May" and the two leaders also discussed a range of other issues, officials said.